Answer a career chance card wrong always makes my sim angry!
No honestly you can try the mischievous to get them irritated. Look at your conversation bar at the top and it should turn orange/red with, don't quote me here, I believe uncomfortable conversation, then do mean interactions till you get them angry. My sim did that on their own but I believe the sim they were harassing was a hot headed sim to begin with.
Hope you can get someone angry!
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No honestly you can try the mischievous to get them irritated. Look at your conversation bar at the top and it should turn orange/red with, don't quote me here, I believe uncomfortable conversation, then do mean interactions till you get them angry. My sim did that on their own but I believe the sim they were harassing was a hot headed sim to begin with.
Hope you can get someone angry!